CloudLinux's Cagefs allows each user to have their own custom php.ini settings with the php selector. However the options presented inside have pre-defined limits that may not work for all users.
It is possible to modify custom settings by hand through the command line.
Start by going into the command line. After you're in, run the following command to get into the specific user's caged environment:
cagefsctl -e <username>
This will take you to a new prompt. Once there, you can use a text editor to modify the php settings directly:
nano /opt/alt/phpXX/link/conf/alt_php.ini
Once there, you will see a section like this:
;>=== Start of PHP Selector Custom Options === ;<=== End of PHP Selector Custom Options =====